Framework stabilization of Si-rich LTA zeolite prepared in organic-free media.

نویسندگان

  • Marlon T Conato
  • Matthew D Oleksiak
  • B Peter McGrail
  • Radha K Motkuri
  • Jeffrey D Rimer
چکیده

Zeolite HOU-2 (LTA type) is prepared with the highest silica content (Si/Al = 2.1) reported for Na-LTA zeolites without the use of an organic structure-directing agent. The rational design of Si-rich zeolites has the potential to improve their thermal stability for applications in catalysis, gas storage, and selective separations.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Controlled Crystallization of LTA Zeolitic Nanoparticles from a Clear Solution Using Organic Template

LTA Zeolite nanoparticles was successfully synthesized from clear solution under controlled conditions using hydrothermal method using tetramethyl ammonium hydroxide as a structural directing agent. The as-synthesized LTA zeolite particles were characterized by powder X-ray Diffraction (XRD) analysis, Scanning Electron Microscopy (SEM), Fourier Transform InfraRed (FT-IR) spectroscopy, </e...

متن کامل

Periodic modeling of zeolite Ti-LTA.

We have proposed a combination of density functional theory calculations and interatomic potential-based simulations to study the structural, electronic, and mechanical properties of pure-silica zeolite Linde Type A (LTA), as well as two titanium-doped compositions. The energetics of the titanium distribution within the zeolite framework suggest that the inclusion of a second titanium atom with...

متن کامل

Preparation and characterization of template-free mordenite type zeolite and comparison of m-xylene isomerization reaction over mordenite and SAPO-11

In this work, Mordenite zeolite was successfully synthesized with Si/Al ratio of 18 in absence of organic template. The hydrothermal method was applied for synthesis under optimum conditions: 24 h synthesis time, 180°C temperature and 2 days aging time. The obtained zeolite was characterized by X-ray powder diffraction (XRD), Brunauer-Emmett-Teller (BET), X-ray fluorescence (XRF), Fourier Trans...

متن کامل

Preparation and characterization of template-free mordenite type zeolite and comparison of m-xylene isomerization reaction over mordenite and SAPO-11

In this work, Mordenite zeolite was successfully synthesized with Si/Al ratio of 18 in absence of organic template. The hydrothermal method was applied for synthesis under optimum conditions: 24 h synthesis time, 180°C temperature and 2 days aging time. The obtained zeolite was characterized by X-ray powder diffraction (XRD), Brunauer-Emmett-Teller (BET), X-ray fluorescence (XRF), Fourier Trans...

متن کامل

Organic-free synthesis of zincoaluminosilicate zeolites from homogeneous gels prepared by a co-precipitation method.

Zeolites containing Zn in their frameworks are promising materials for ion-exchange and catalysis because of their unique ion-exchange capabilities and characteristic Lewis acidity. However, expensive organic compounds often required in their synthesis can prevent their practical uses. Here, a facile organic-free synthesis route for new zincoaluminosilicate zeolites having MOR topology, in whic...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:
  • Chemical communications

دوره 51 2  شماره 

صفحات  -

تاریخ انتشار 2015